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Collect. Czech. Chem. Commun. 1998, 63, 1498-1512
https://doi.org/10.1135/cccc19981498

Generation and Reactivity of Chromium Fluoride Cations (CrF+n, n = 0-4) in the Gas Phase

Ulf Mazurek, Detlef Schröder and Helmut Schwarz

Institut für Organische Chemie, Technische Universität Berlin, Strasse des 17. Juni 135, D-10623 Berlin, Germany

Crossref Cited-by Linking

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  • Zhao Jin, Qi Lingxi, Li Wenzuo, Cheng Jianbo, Li Qingzhong, Liu Shaoli: CH4 activation by PtX+ (X = F, Cl, Br, I). Front. Chem. 2022, 10. <https://doi.org/10.3389/fchem.2022.1027465>
  • Yan Linghui, Li Shihan, Zhou Shaodong: On the origin of reactivity variation upon sequential ligation: the [Re(Cl)x]+/CH4 (x = 1–3) couples. Phys. Chem. Chem. Phys. 2021, 23, 24319. <https://doi.org/10.1039/D1CP03468E>
  • Chen Qiang, Zhao Yan-Xia, Jiang Li-Xue, Li Hai-Fang, Chen Jiao-Jiao, Zhang Ting, Liu Qing-Yu, He Sheng-Gui: Thermal activation of methane by vanadium boride cluster cations VBn+ (n = 3–6). Phys. Chem. Chem. Phys. 2018, 20, 4641. <https://doi.org/10.1039/C8CP00071A>
  • Zhou Shaodong, Li Jilai, Schlangen Maria, Schwarz Helmut: Thermische Aktivierung von Methan durch [HfO].+ und [XHfO]+ (X=F, Cl, Br, I): ein außergewöhnlicher Ligandeneffekt und dessen Ursache. Angewandte Chemie 2016, 128, 7816. <https://doi.org/10.1002/ange.201602312>
  • Zhou Shaodong, Li Jilai, Schlangen Maria, Schwarz Helmut: Thermal Activation of Methane by [HfO].+ and [XHfO]+ (X=F, Cl, Br, I) and the Origin of a Remarkable Ligand Effect. Angew Chem Int Ed 2016, 55, 7685. <https://doi.org/10.1002/anie.201602312>
  • Zhao Lianming, Ding Qiuyue, Xu Wenbin, Sang Pengpeng, He Xiaoli, Shi Zemin, Chi Yuhua, Lu Xiaoqing, Guo Wenyue: The ligand effect on the selective C–H versus C–C bond activation of propane by NiBr+: a theoretical study. Theor Chem Acc 2015, 134. <https://doi.org/10.1007/s00214-015-1628-4>
  • Schwarz Helmut: How and Why Do Cluster Size, Charge State, and Ligands Affect the Course of Metal‐Mediated Gas‐Phase Activation of Methane?. Israel Journal of Chemistry 2014, 54, 1413. <https://doi.org/10.1002/ijch.201300134>
  • Gholami Ameneh, Fridgen Travis D.: Dehydrogenation and demethanation of 2-methylpropane and propane in the gas-phase by the 16-electron complex [Ru(bipy)2(CO)]2+* chemically activated by the association of [Ru(bipy)2]2+ and CO. Dalton Trans. 2013, 42, 3979. <https://doi.org/10.1039/c2dt32475j>
  • Roithová Jana, Schröder Detlef: Selective Activation of Alkanes by Gas-Phase Metal Ions. Chem. Rev. 2010, 110, 1170. <https://doi.org/10.1021/cr900183p>
  • Schlangen Maria, Schwarz Helmut: Ligand and electronic-structure effects in metal-mediated gas-phase activation of methane: A cold approach to a hot problem. Dalton Trans. 2009, 10155. <https://doi.org/10.1039/b915165f>
  • Schröder Detlef, Schwarz Helmut: Gas-phase activation of methane by ligated transition-metal cations. Proc. Natl. Acad. Sci. U.S.A. 2008, 105, 18114. <https://doi.org/10.1073/pnas.0801849105>
  • Schlangen Maria, Schröder Detlef, Schwarz Helmut: Ligand and Substrate Effects in Gas‐Phase Reactions of NiX+/RH Couples (X=F, Cl, Br, I; R=CH3, C2H5, nC3H7, nC4H9). Chemistry A European J 2007, 13, 6810. <https://doi.org/10.1002/chem.200700506>
  • Antoniotti Paola, Rabezzana Roberto, Turco Francesca, Borocci Stefano, Bronzolino Nicoletta, Grandinetti Felice: Gas-phase ion chemistry of NF3/SO2 mixtures: A mass spectrometric and theoretical investigation. International Journal of Mass Spectrometry 2007, 266, 86. <https://doi.org/10.1016/j.ijms.2007.07.011>
  • Zhao Xiang, Koyanagi Gregory K., Bohme Diethard K.: Reactions of Methyl Fluoride with Atomic Transition-Metal and Main-Group Cations:  Gas-Phase Room-Temperature Kinetics and Periodicities in Reactivity. J. Phys. Chem. A 2006, 110, 10607. <https://doi.org/10.1021/jp062625a>
  • Kretzschmar Ilona, Schröder Detlef, Schwarz Helmut, Armentrout P.B.: Structure, thermochemistry, and reactivity of MSn+ cations (M=V, Mo; n=1–3) in the gas phase. International Journal of Mass Spectrometry 2003, 228, 439. <https://doi.org/10.1016/S1387-3806(03)00137-4>
  • Mazurek Ulf, Koszinowski Konrad, Schwarz Helmut: C−F Bond Activation in Fluorinated Carbonyl Compounds by Chromium Monocations in the Gas Phase. Organometallics 2003, 22, 218. <https://doi.org/10.1021/om020646v>
  • Mazurek Ulf, Schröder Detlef, Schwarz Helmut: Gas-Phase Reactions of Chromium and Chromium Fluoride Cations CrFn+ (n = 0−4) with Water and Nitrous Oxide. Eur J Inorg Chem 2002, 2002, 1622. <https://doi.org/10.1002/1099-0682(200207)2002:7<1622::AID-EJIC1622>3.0.CO;2-V>
  • Mazurek Ulf, Schröder Detlef, Schwarz Helmut: Gas-Phase Reactions of Chromium and Chromium Fluoride Cations CrFn+ (n = 0−4) with Water and Nitrous Oxide. Eur. J. Inorg. Chem. 2002, 2002, 1622. <https://doi.org/10.1002/1099-0682(200207)2002:7<1622::AID-EJIC1622>3.0.CO;2-V>
  • Mazurek Ulf, Schröder Detlef, Schwarz Helmut: Hydrolytic Activation of CF Bonds in the Gas Phase by Intrinsically Unreactive Chromium Cations. Angew Chem Int Ed 2002, 41, 2538. <https://doi.org/10.1002/1521-3773(20020715)41:14<2538::AID-ANIE2538>3.0.CO;2-4>
  • Mazurek Ulf, Schröder Detlef, Schwarz Helmut: Hydrolytic Activation of CF Bonds in the Gas Phase by Intrinsically Unreactive Chromium Cations. Angew. Chem. Int. Ed. 2002, 41, 2538. <https://doi.org/10.1002/1521-3773(20020715)41:14<2538::AID-ANIE2538>3.0.CO;2-4>
  • Schröder Detlef, Trage Claudia, Schwarz Helmut, Danovich David, Shaik Sason: Inner-sphere electron transfer in metal-cation chemistry. International Journal of Mass Spectrometry 2000, 200, 163. <https://doi.org/10.1016/S1387-3806(00)00349-3>
  • Mazurek Ulf, Schwarz Helmut: Gas-Phase Reactions of Chromium and Chromium Fluoride Cations CrFn+ (n = 0−4) with Phosphane. Inorg. Chem. 2000, 39, 5586. <https://doi.org/10.1021/ic000318s>
  • Gapeev Alexei, Dunbar Robert C.: Binding of Alkaline Earth Halide Ions MX+ to Benzene and Mesitylene. J. Phys. Chem. A 2000, 104, 4084. <https://doi.org/10.1021/jp9943934>
  • Harvey Jeremy N., Diefenbach Martin, Schröder Detlef, Schwarz Helmut: Oxidation properties of the early transition-metal dioxide cations MO2+ (M = Ti, V, Zr, Nb) in the gas-phase. International Journal of Mass Spectrometry 1999, 182-183, 85. <https://doi.org/10.1016/S1387-3806(98)14241-0>